A Water-Borne Adhesive Modeled after the Sandcastle Glue of P. californic
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A Water-Borne Adhesive Modeled after the Sandcastle
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PolyacrylateglueproteinanalogsofthegluesecretedbyPhragmatopomacalifornica,amarineposynthesizedwithphosphate,primaryamine,andcatecholsidechainswithmolarratiossimilartothproteins.AqueousmixturesofthemimeticpolyelectrolytescondensedintoliquidcomplexcoacervneutralpH.Wetcorticalbonespecimensbondedwiththecoacervates,oxidativelycrosslinkedthrosidechains,hadbondstrengthsnearly40%ofthestrengthofacommercialcyanoacrylate.Theuniqpropertiesofcomplexcoacervatesmaybeidealfordevelopmentofclinicallyusefuladhesivesandbiomaterials.
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